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I love WataMote's OP myself too. I also love Rising Hope too - ugh, can't stop listening to that OP. Like GabbyHeart and GeneralOtter, I have a lot myself too. Too many to point out. In terms of instrumental tracks, I mostly dig Madoka Magica's soundtrack though. Yuki Kajiura is a master. On the non-instrumental side, I actually made a whole list of my favorite OPs and EDs on my MAL profile: Opening A Certain Scientific Railgun Black Lagoon Blue Exorcist Bokurano DanganRonpa: Academy of Hope and High School Students of Despair - The Animation Darker Than Black: The Black Contractor HOWLING Deadman Wonderland Digimon Tamers Fate/Stay Night ~Realta Nua~ , Fullmetal Alchemist: Brotherhood , Rain Ga-Rei Zero Gintama , Highschool of the Dead Higurashi no Naku Koro ni Naraku no Hana, , Hourou Musuko Kino's Journey Mahouka Koukou no Rettousei Rising Hope Mirai Nikki Nichijou , One Piece Paranoia Agent Pocket Monsters Mezase Pokémon Master, OK!, Ready Go!, Advance Adventure, , , Together Pokémon (English Dub) Rewrite Shiki , The Melancholy of Haruhi Suzumiya , WataMote Ending Bokurano , Detective Conan , Secret of My Heart, Summer Memories, , Your Best Friend, Kimi e no Uso Digimon Tamers Fairy Tail Gintama Genjou Destruction Higurashi no Naku Koro ni , Hourou Musuko K-On Don't say "lazy", NO, Thank You! Little Busters! Mirai Nikki Paranoia Agent Pocket Monsters , Type: Wild, Maemuki Rocket-dan!, Polka O Dolka, The Melancholy of Haruhi Suzumiya Welcome to the NHK! , You can click on the links above if you wanna listen to them (most of them are dead links, I would presume), but I'm too lazy to post all of their YouTube clips, and I don't want to spam the page with many videos, so I'm just gonna post some here:

I would have liked the one with Nanoha, however it seems you were right to call browser crash, as when I tried to load it, the browser started to choke !